Synthesis of Cadmium Oxide and its
Transcription
Synthesis of Cadmium Oxide and its
Advanced Materials Research Vol. 678 (2013) pp 369-372 © (2013) Trans Tech Publications, Switzerland doi:10.4028/www.scientific.net/AMR.678.369 Synthesis of Cadmium Oxide and its Electrochemical Detection of Pollutants K.Giribabu1, R. Suresh1, L. Vijayalakshmi2, A. Stephen3 and V. Narayanan1* 1 Department of Inorganic Chemistry, University of Madras, Guindy Campus, Chennai 600025 Tamil Nadu, India 2 CSI Ewart Women’s Christian College, Melrosapuram, Kancheepuram 603204 Tamil Nadu, India 3 Department of Nuclear Physics, University of Madras, Guindy Campus, Chennai 600025 Tamil Nadu, India a [email protected], [email protected] [email protected], d [email protected], e*[email protected] Keywords: CdO, Electrocatalyst, 4-Nitrophenol, 2-Nitrophenol Abstract. Cadmium oxide was synthesized using cadmium acetate and oleic acid as the precursor and capping agent, the main role of oleic acid to cap the formed cadmium oxide and to control the particle size. The formed cadmium oxide nanoparticles were characterized by using FT-IR, XRD,FE-SEM and cyclic voltammetry. The electrochemical detection of pollutants (4-Nitrophenol and 2-Nitrophenol) was carried out by coating the cadmium oxide onto the glassy carbon electrode (GCE) by drop coating method. The electrocatalytic performance of the modified GCE electrode was best with 4-Nitrophenol. In case of 2-Nitrophenol the electrocatalytic performance was not observed but increase in current response indicates the ability of modified electrode to be a useful one for sensing the environmental pollutants. 1. Introduction Cadmium oxide (CdO) is a n-type II–IV semiconductor with a direct band gap of 2.5 eV and an indirect band gap of 1.98 eV [1]. The unique combination of high electrical conductivity, high carrier concentration and high transparency in the visible range of electromagnetic spectrum has prompted its optoelectronic applications. Recently, CdO nanostructures have been synthesized in different interesting morphologies including nanowires, nanotubes, nanofibers, nanorods, nanoclusters, nanocubes, and nanobelts by different methods like hydrothermal method, template assisted method, solvothermal methods, chemical co-precipitation method vapor phase transport, thermal evaporation and sonochemical method etc., [2-3]. 4-Nitrophenol (4-NP) and 2-nitrophenol (2-NP) is included in the US Environmental Protection Agency List of Priority Pollutants . 4-NP is a hazardous substance that can have a major environmental impact due to its toxicity and persistence. Hence, the determination of 4-NP is of great importance, and various methods have been developed. Chromatographic methods [4] are commonly used to detect 4-NP and 2-NP. Recently, electrochemical techniques based on various chemically modified electrodes [5-6] have been published to detect 4-NP. Here we report the synthesis of CdO using oleic acid as the surfactant and cadmium acetate as the cadmium source. The as-synthesized CdO have employed for the sensing towards the 4-NP and 2-NP. 2. Experimental 2.1 Reagents Cadmium acetate, Oleic acid, sodium hydrogen phosphate and sodium dihydrogen phosphate were purchased from Qualigens and used as received. 4-Nitrophenol and 2- Nitrophenol were purchased from CDH, India. Other chemicals used were of analytical reagent grade. All chemicals were used without further purification. All rights reserved. No part of contents of this paper may be reproduced or transmitted in any form or by any means without the written permission of TTP, www.ttp.net. (ID: 14.139.186.162, University of Madras, Chennai, India-16/03/13,10:54:57) 370 Advances in Nanoscience and Nanotechnology 2.2 Synthesis of CdO nanoparticle 1.33 g of cadmium acetate was dispersed in 12 mL hot oleic acid and stirred well. After the formation of white precipitate the mixture was kept in an oil bath. The oil bath temperature was maintained at 140 oC for 3 h. To remove oleic acid, the resulting suspension was washed with hot ethanol three times. Further, the sample was pyrolysed at 450 oC for 3 h. 2.3 Characterization FTIR spectroscopy of the CdO was studied using Schimadzu FTIR 8300 series instrument. The phase and structure of CdO was analyzed by a Rich Siefert 3000 diffractometer with Cu-Kα1 radiation (λ = 1.5418 Å). The electrochemical experiments were performed on a CHI 600A electrochemical instrument using the as-modified electrode and bare GCE as working electrode, a platinum wire was the counter electrode, and saturated calomel electrode (SCE) was the reference electrode. 2.4 Preparation of CdO Coated GCE CdO coated GCE was prepared by following the literature method [7, 8] as follows.The CdO suspension was prepared by dispersing a 5 mg CdO in 10 mL of distilled ethanol during 20 min of ultrasonic agitation. Prior to modification, the GCE was mechanically polished with alumina paste of different grades to mirror finish, rinsed, and sonicated in redistilled water for 2 min. Finally, the GCE was coated with 10 µL of the suspension and dried in air. 3. Result and discussion 3.1 XRD, FE-SEM and FTIR studies The XRD pattern of CdO (Fig. 1) shows the diffraction peak that matches with standard file card (JSPDCS.05-0640). It was observed that the diffraction peaks of CdO show narrow peaks indicating the agglomerated particles of the sample. The FTIR spectrum of CdO is shown in Fig. 2. The spectrum exhibits a common broad band near 3400 cm−1 due to the OH-stretching vibrations of free and hydrogen-bonded hydroxyl groups. The band at 580, 968 and 1400 cm−1 [9, 10, 11] are characteristic of CdO. The FE-SEM images clearly indicates the formation of nanoparticles in the range of 200-250 nm of shown in Fig.3. Fig. 1 XRD pattern of CdO nanoparticles Fig. 2 FTIR spectrum of CdO nanoparticles Fig. 3 FE-SEM images of CdO nanoparticles Advanced Materials Research Vol. 678 371 3.2 Electrocatalytic property Fig. 4 shows the electrooxidation of 1- 5 mM 4-NP for CdO modified GCE at +0.69 V in 0.1 M PBS (Phosphate buffer solution) as the electrolyte. Bare GCE shows a broad oxidation peak at+ 0.81 V. The modified GCE shows an oxidation peak with higher current response than the bare GCE. Hence it is clear that the oxidation potential for 4-NP at the modified electrode was shifted to less positive direction than the bare GCE, and the 4-NP oxidative current was largely increased relative to the bare GCE, indicating the electro catalytic ability of the CdO modified electrode. Fig.5 shows effect of scan rate of the modified electrode in 1mM 4-NP. When increasing the scan rates from 50-250 mVs-1 the anodic peak current increases, which is an indicative of the process is purely diffusion-controlled process. The reason for the electrocatalytic property is the large surface area when compared to that of the bare electrode, hence the electrocatalytic behavior of the modified electrode was found to be more active for the sensing of 4-NP. . Fig. 4 Cyclic voltammogram of (a) bare and CdO modified GCE for different Concentrations of 4-NP (b-f: 1-5mM) at 50 mV s-1 Fig. 5 Plot of square root of scan rate vs. current response Fig. 6 shows the electrooxidation of 1-5 mM 2-NP for CdO modified GCE at +0.79 V in 0.1 M PBS as the electrolyte. Bare GCE shows a broad oxidation peak at +0.78. With lower current response when compared to that of modified electrode. Fig.7 shows effect of scan rate of the modified electrode in 1mM 2-NP. When increasing the scan rates from 50-250 mVs-1 the anodic peak current increases, which is an indicative of the process is purely diffusion controlled process. The reason or the electrocatalytic property is the large surface area when compared to that of the bare electrode, hence the electrocatalytic behavior of the modified electrode was found to be more active for the sensing of 2-NP. Fig. 6 Cyclic voltammogram of (a) bare and CdO modified GCE for different Concentrations of 2-NP (b-f: 1-5mM) at 50 mV s-1 Fig. 7 Plot of square root of scan rate current response 372 Advances in Nanoscience and Nanotechnology 4. Conclusion Cadmium oxide nanoparticles were synthesized by two step procedure involving simple steps. The synthesized nanoparticles have employed to modify the GCE to evaluate the electrocatalytic performance towards environmental pollutants such as 4-NP and 2-NP. The electrocatalytic performance was good with 4-NP with respect to the oxidation potential when compared with bare GCE and for 2-NP the performance was found to be moderate, since increase in current response alone observed not in shifting of the potentials. Acknowledgment: The authors (KG) wish to acknowledge DST for their financial assistance in the form of INSPIRE fellowship (Inspire fellow IF 10226) under ‘Assured Opportunity for research career (AORC)’and NCNSNT, University of Madras for recording FE-SEM images. References [1] M. Ortega, G. Santana, A. Morales-Acevedo, Solid State Electron., Optoelectronic Properties of CdO/Si Photodetectors 44 (2000) 1765-1769. [2] T.P. Gujar, V.R. Shinde, W.Y. Kim, K.D. Jung, C.D. Lokhande, O. Joo, Formation of CdO films from chemically deposited Cd(OH)2 films as a precursor Appl. Surf. Sci., 254 (2008) 3813-3818. [3] T. Kuo, M.H. Huang, Gold-Catalyzed Low-Temperature Growth of Cadmium Oxide Nanowires by Vapor Transport J. Phys. Chem. B, 110 (2006) 13717-13721. [4] R. Belloli, B. Barletta, E. Bolzacchini, S. Meinardi, M. Orlandi, B. Rindone, Determination of toxic nitrophenols in the atmosphere by high-performance liquid chromatography J. Chromatogr. A, 846 (1999) 277–281 [5] D. Puig, I. 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